Published In

Applied Physics Letters

Document Type

Article

Publication Date

2-1-2017

Subjects

Magnetization, Lithium cells, Iron oxides, Electric fields, Stoichiometry

Abstract

In this report, a reversible control of Fe₃O₄ saturated magnetization by Li ions is demonstrated. A miniature Li ion battery (LIB) was assembled using a Fe₃O₄ nanoparticle layer as the active cathode. A stable magnetism modulation is realized by a nondestructive electrochemical process in which the lithium insertion results in a valence change and partial redistribution of Fe cations in the crystal structure. The relation between the discharge voltage and the chemical phases were studied by ex situ X-ray diffraction and magnetic measurement. In a suitable discharge potential range, a reversible control of Fe₃O₄ saturated magnetization was obtained without structural damage to the magnetic electrode. The experimental results indicate by further optimizing the LIB's performance, a large reversible change in magnetization could be realized at room temperature, suggesting the potential for future practical applications.

Description

This article is licensed under a Creative Commons Attribution 3.0 Unported Licence. http://creativecommons.org/licenses/by/3.0/

DOI

10.1063/1.4975773

Persistent Identifier

http://archives.pdx.edu/ds/psu/19503

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